Heterogenous Photochemical Electron Transfer
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A01=Michael Gratzel
annihilation
Author_Michael Gratzel
Band Gap
Category=PHVQ
charge
Charge Carrier
Charge Carriers
Charge Transfer
charge transfer kinetics
Colloidal Semiconductors
Colloidal TiO
Conduction Band
Conduction Band Electrons
constant
Electron Hole Pairs
Electron Transfer Rate Constant
Electron Transfer Reactions
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events
Flat Band Potential
induced
Interfacial Electron Transfer
light
Light Harvesting Unit
Light Induced Charge Separation
Micellar Assemblies
Micellar Surface
Nonadiabatic Electron Transfer
organized molecular assemblies
Photoinduced Electron Transfer
photoinduced electron transfer in micelles
quantum size effects
rate
reactions
redox processes
Reorganization Energy
Self-exchange Reaction
Semiconductor Electrode
semiconductor interfaces
Semiconductor Particle
separation
solar energy conversion
Space Charge Layer
triplet
Triplet Triplet Annihilation
Product details
- ISBN 9781315894102
- Weight: 470g
- Dimensions: 178 x 254mm
- Publication Date: 29 Nov 2017
- Publisher: Taylor & Francis Ltd
- Publication City/Country: GB
- Product Form: Hardback
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The present monograph attempts to unify these diverse and exciting new developments within a common framework. First, the physical principles underlying heterogenous electron-transfer processes are outlined in a concise way and are compared to the homogeneous counterpart. This analysis includes the notion of the Fermi level in liquids and solids as well as the distribution of electronic energy levels in solids and liquids. A comparison is made between the salient kinetic features of homogeneous and heterogeneous electron transfer reactions. This establishes the basis for the subsequent treatment of the transduction of excitation energy and photo-initiated electron transfer in organized molecular assemblies, such as micelles, vesicles and monolayers. Transmembrane redox processes are critically reviewed. Particular attention is given to semiconductor electrodes and particles. This includes a discussion of quantum size effects, the nature of space charge layers as well as surface states and the dynamics of charge carrier-induced redox reactions at the semiconductor solution interface. These processes are of fundamental importance in such diverse fields as photochromism, electrochromic displays, electroreprography and photography, information storage, photocatalysis, photodegradation of paints, and solar energy conversion.
